Investigation of Nuclide Importance to Functional Requirements Related to Transport and Long ...

123 Pages·02.25 MB·English

ORNL/TM-12742
Investigation of Nuclide Importance
to Functional Requirements
Related to Transport and
Long-Term Storage of LWR
Spent Fuel
B. L. Broadhead
M. D. DeHart
J. C. Ryman
J. S. Tang
C. v. Parks
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Government or any agency thereof.
ORNL/TM-12742
Computational Physics and Engineering Division
INVESTIGATION OF NUCLIDE IMPORTANCE TO FUNCTIONAL
REQUIREMENTS RELATED TO TRANSPORT AND LONG-TERM
STORAGE OF LWR SPENT FUEL
daehdao r..BLB
M. D. DeHart
n. aJ.mCyR
J. S. Tang
C. V. Parks
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TABLE OF CONTENTS
Page
LIST OF FIGURES ............................................................... vi
LIST OF TABLES ................................................................ v
TCARTSBA .................................................................... iiv
1. INTRODUCTION ............................................................. 1
.2HC AORPPA ................................................................. 3
2.1 AREAS OF INTEREST .................................................. 3
DO HST IE2SM.Y2 LANA .................................................. 3
.3 STLNUO SIDESNRSAUCSID ................................................... 5
SG N YI YTK1TEN.IFA3LARAS CITIRC ...................................... 5
SGN I GK2NN.IA3DR LEIHS ................................................ 9
S G3N.I 3KE NIARRUC ................................................... 14
SGNIK NTA ARY4EA.H C3ED ............................................. 14
SGNI KYNTAIRC ILXAOCTIG O5L.O3 IDAR ................................. 17
YR A6M. M3US .......................................................... 21
.4 SNOISULCNOC ............................................................. 25
5. REFERENCES .............................................................. 26
XIDNE P.PAA Y TYIT LESAFTCAOISLTPIRC ...................................... 29
XIDNEPPA .B ESOD ETAR NOITCARFSTOLP ..................................... 49
XIDNEPP A.C EIRU CL ENVOEILTCSATROFLP .................................... 81
XID N.EDPPA NYSO ATITCOTAELCEDPAHRF .................................... 89
XI DNN OEYS. IPTTELTPIOACACLCAIPIRXGF OOTLOIDAR ........................ 97
iii
LIST OF FIGURES
Figure Page
1 kn ogniloo cmret-gno lf otceffE . .............................................. 8
4
iv
LIST OF TABLES
Table Page
1 rieh tdn aseidut sgnikna rn ides usnoitanibmo ctnemhcirn edn apunruB
spunr uebgare vyartsud nositpihsnoitaler ......................................... 4
2 snoitpros blaat o f t%on1a hrtetae rhgt iswedinit c fasogniknaR
ta 5 d n0a00s,r0a3ey ....................................................... 6
3 tsanoitpros blaat of%to1 .n0a hrtetae rhgt iswtcudo rnpoiss ifsfogniknaR
s r0 a0 5e0dy,n0a3 ......................................................... 7
4 kf onosirapmo cdn aseitivitisne sedinitcA sgnikn anroitprosba-sv- .................... 10
ffe
5 fknoosirapm odc nsaeitivitisn etscudorp-noissiF sgnikn anroitpros bda na .............. 11
ffe
6 teas oldat o ft %on1a hrtetae rhgt iswedinit c fasognikn agrnidleihS
s r0 a0 5e0dy,n0a1 ........................................................ 12
7 % 1nah tretaer ghti wstnemel ethgi ldn astcudor pnoissi ff osgnikna rgnidleihS
em igtnilo orcaey - ta5eas oldat ofto ........................................... 12
8 ht iswtneme ltehg idl n,astcudo rnpoiss i,fsedinit c fasognikn aeriruC
sr a0 se0tey0 ai ,d5rl 0nua %1 actf1n oo.art0hettaerg ............................. 15
9 stneme ltehg idl n,astcudo rnpoiss i,fsedinit c fasognikn atra eyhaceD
sra e0y00, 0d tt1n5aa aeyhac eldat of%nto1a hrtetae rhgtiw ........................ 16
10 noissi fdn a,sedinitc a,stnemel ethgi lf osgnikna ryticixo tnoitsegnI
evitcef fdeettimm olcaitnet olpat o ft%o1 .n0a hrtetae rhgt iswtcudorp
sra e0y00, 0d 1 nt5taanelaviu qeesod ........................................... 18
11 stcudo rnpoiss idf n,asedinit c,astneme ltehg i flsognikn ayrticix ontoitalahnI
tnelaviuq eeso devitceff edettimmo claitneto plato tf o%1. 0nah tretaer ghtiw
ta 5 d n0a00s,r0a1ey ....................................................... 19
12 )sedinitc aa(e rsaisyla n yasbgnikn ayrrammuS ................................... 22
13 )stneme ltehg idl nsatcudo rnpoissi fs(ae rsaisyla n yasbgnikn ayrrammuS ............... 23
14 sdoht elmacityla ntanerr u fcyotilibacilp pda nyacaruccA ............................ 24
v
vi
ABSTRACT
Tilcunoidar eh ngis eed h ntsiel oyr eyka llpe utfne p)sRW Lr(otcaer-retaw-thg i flsocitsiretcara hecd
and l , dsaenenhaiittfil iecgaa frmoitr se,tsnmie tnsoyistatrops ne atersvtaiwtca o siredoiaftriv igtnciasneci l
na fo saera lareveS .ertis yrotisope roivahe btnedneped-emi teh tgninrecno cnoitamrofn ideliate deriuqe rsisyla
of radi yesaber rc -,org a ssungmreb oi nmoiassd eiafd/el)vdgued e2iu/tli)i(tlnsil1hccosc(sanrsuoitinufen r
conce snoitartn rof ytilacitirc ytefas ,snoitanimreted )3( laudiser yaced taeh snoitciderp rof amreht l
,snoitaredisnoc dna e hott ndiesael e er obdtemus ssalairet arm osflev eylticix oltacigoloid arro/d neair u)c4(
tnemnorivne/dnuorg . e smfdiooti rg enrpoe ltfa ht orbe vsonoitcide repdilcunoid aer h fteorut alnaicu rec hT
edilcunoida rro fnoitadila vhguoroh tn osisahpm edesaercn in an idetluse rsa hemi tf osdoire pgno ldn atrohs
.sedo cnoitelped/noitareneg
tnerruC wol lyoottfiliba p eaeh cvtsaeh dnoocitelped/noitare needgilcunoi dar emo sf onoitulov eeht
1600 sep ogtnoi srniu odhittoabi ddanrar iyaced e m.istdoirep fO ,yelsleahc tiyplynto 01 ot 02edilcun s
ar evitatitnauq a suhT .aera sisylana hcae ot snoditubirtnoc etanimo sdoire pemi tsuoira vrev osedilcu nf ognikn
si derised rof hcae fo eht sisylana saera fo ,gnidle i,hystilacitirc taeh ,refsnart dna latnemnorivnesod e
dluohs sgniknar esehT .)yticixot l(acigoloidar desuco fe bo tstroff etnemevorpm iata ddn anoitadila vro fwolla
.sedilcu ntnatropm itso meh tn oylno
This study ,t cdtunhdagoirlp- n so,eiecs dns fiaiso n tfuesierovetho iitctpertaamhaagitvli etrsevni -
emele tn sepotosi detaicossa htiw RWL tneps leuf htiw tcepser ot evif sisylana :saera ytilacitirctefas y
itc(arf noitprosba fnooitcar ft(a eyhac e,d)slev esleir ulcanoitcar fs(eir u,c)snoitca reft aerso dg(nidlei h,s)sno
to tal ,)sttaw dlnaaci gyotlio cinidoxaiorttcarf( fo lai tdneett toeipvmimtocceff e e.s)otdnelaviuqe sehT e
ra sgnikn era detneserp rof pu ot txnie sm shtocniierrranenefe/fcpisu dndrnuab ta yaced semit morf 2t o
1aR .sraey 000,00 s,assenetelpm orc oxfidnep p nA naniev ieg rsaae rsaisyla nease h fthoc are osfto lgpnikn
llew as sum syerl abnmai te hn tiy addmo ebf.st o tg nnser neeimhoyirsr tp rkaeefeanrtormapgmriuhS h
%0(1 naht retaerg na hstse lw( odl n,a)noitubirtn o%c 0d1 n %an1eewte bm(uid e,m)lat oet h otntoitubirtn oc
1% contri )n o.rig otnm-hfuirttnble r o eotdodbmo-n he ec gahsrnrdntaeueo iphstlewmWachoeetcmpxe t
,seicarucca es eht e hrt oyfltneiciff udseziretcara h ecnb ascepoto stinatrop mei h fttos otma hwto hssgniknar
pidar fo esopru nia meh tesuac e .Bsaer asisylan aeh tf ohca en inoitadila vedo cnoitelped/noitarene gedilcuno
epotosi fo secnatropmi evitaler eht no si krow fsiht fo suco snoisulcn oecm o,sle utfne pRs WhLt idwetaicos ssa
may not eelbbacil popt arali msiasera hcus lseave le-thsga iw)ghtWnnLieHrn(ao epdbmn-oalceufnon s
.)CBFN(
vii
1. INTRODUCTION
The Depart tnem f os'yg r)eEnOE De(ciffO fe ovniati clteaintovesiimadaCeWargRgaonraPM m
)MWRCO( ytcc iAel torsPaae W lheecthcuitnNwad r, odnceichasilb astaswe da eel h steavr e os,t28 9f1o
itcurtsnoc ,gonitis )1( rof eciff tne plsaicremm ogcnitropsna r)t 2,(seirotisop eerts arwaelc ugnnitare pdo n,agn
nuclear f l e lu,e s vgedentn lisa)-pa3how( gl lieaahvse odt p ceooulrgtrbpa tardsv oeneatroisocrttienrom e
facilit ,y dil c ntu.ou nsioeom tb hi esa a tdele mgt agbi rnndlra otnoiene rgriifvpau)onplnlsf4tiiIo(sdtsiua e
hc are oyfrassec e snsiema refm ittnereff igdnir usdets alwevel-hg idh nlae utfne pssuoir a fvsocitsiretcarahc
. sae rkar oewse hfto
EOD eTht ,deen siht teem o edivo r op)tBD Ce(s aaBt acDitsiretcara heC hdtepolev esd aMhWRCO-
margorp stnapicitrap ,snoisnem i,dseititna ueq httuo bnaoitamrof n fieocru odseifila udq ntanetsisn ohactiw
oidar dna ,etsaw level-hgih ,leuf tneps fo asnoitisopmoc dn e. hsTtnenopm orcotca erraelc ulnaicremm oecvitca
CDB (cu y pd orecamhulo v d-fer osuai or nfp )oms1ioisci vyelrtnerr 1 troper dna xis atad sesab taht nacb e
dessecca r.e) tC luPap( nmaooiscvrep sa hdn a,weive rree placinhce tevisnetx en aenogredn usa hBD CehT
a ytilauq" ni esu rof MWRCO ybb "deifitrec" nee xi seh tf oe n .Omargor pMWRC Oeh tnihti wkro w"gnitceff
aB ataD lacigolodidaR eht si sesab ata ,ta eyhac e,dseir u,csnoitisopm ohct iswre ssuedivo rdp n)aBDDA Re(s
ruos nortuepn dna ,ecruos notoh -gnili o rb)oRW Pr(otca erretaw-dezirusser pr[otca e freop yet h ntdoes a,bec
mit gnilooc dna ,punrub ,tnemhcirne laiwtini ,])RWB( rotcaer reta mo rdfetae rsc aBwDD A eR. hlTe uef h fteo
IRO meht fo snoitacilppa elpitlu edo cretupmo c2NEG .seirarbi lnoit2ces-ssor cdepoleve dyltnece rgnis u 3 e n O
reep eht fo emoctuo itnatropm ta hetriuq edrlu oBw DeC h ftsonoisiv eerrut utfa hntoitingoc eer hst awweiver
eht MW Rh CtyOilwp ma oteecahtdtar e d noesetsdguoh tseimsyl ana stnemeriuq e)rA Qe(cnarus syatilauq
.erawt froosf
OCRWM formed eht BDC sresU puorG ni lirpA 3991 sa a noissucsid murof rof BDCresU s
ediwnoitan dna ot edi vloarcpinhc ettupni ot pleh ediug erutuf B.DtCnempoleved ynaM fo ehtetrahc r
ocbus ot dengissa erew pumorG sresU BDC eht fo srebme C Pxi seh tf ohca ehti wyllacinhce tdengil aseettimm
g pleh ot dengissa saw eettimmocbus lacigoloiddar ehT .sesab ata dn aBDDA Reh tf otnempoleve drehtru fediu
the verificat noi dna noitadilav stroffe detaler ot eht sisylan a.ygolodohtem ehT laicurc erutan foht e
edilcunoidar dne italu sse seamfdrhiooti rg endtponr laoh htr soesbvnooitcid erp eh tn itseretn idenethgieh
ycarucca fo eht e dniolictuenlopiedda/rnoitar esneedgoc desu ni eht ngised dna ytefas noitaulaveo f
tatropsnar f onoitadila veh t,revew o .Hseitilica fyrotisope retsaw-level-hgi hdn a,egarot smiretn i,metsy snoit
sisylana s ddo eh sst t cuetdcoi mnei tplerdsoe peeituyspr ofbmpys atiedhih e ctarfu tuoataspadahetmra e
avai elbal oitalu cnloaictelped-t nd irdo aepndki ncayaaltrlstac ispeydti l 0c en 0 uevao6enriht1hottt maler n
c eupyt-NEGIRO na gnis elbisso pf oegna rdetimi layln orevo cata dderusae melbaliav aeh t,noitidd an .Iedo
tneps ylbm e,d sengsmanaiit l,otoncemhc ilranie t,ipnuin rsucbi(tsiretca r laehucf tcer ipdl e ohst u. h)Tepyt
future va noitad isltroffe dna tsissa MWRCO ni gniyfitned ieht sedilcun fo ecnatropmi ot ehtanoitcnuf l
,stnemeriuqer eet tfiom mldeoa ehcct d tbi an Bugkhe sDsor tmprCloemue owhooseitcrU bdeGearnrodt o
.sae rsaisyla ntanatrop mri ogfnikn aerdilc uen h fteorusa eemvitatitna ueaqdivorp
T eh,ytilic aefgaro tmsiret n,imets ynsoitatropsna ret h ntsiel oyr eyka lspcitsiretcara hecdilcunoid ar
dna yrot insgoipseerd d ng ansiessnseeccio lrrpof la rseivseysl as nagaenarirad-ualmc mn)ai1g(/nortuen y
sources f ro gnidleih s,seiduts )r2e (bsrnoosibtaa/retlniescsnio fcrof ytilacitir cy t,esfnaositanimreted3( )
snoitciderp taeh yraced laudise r osflev eylticix oltacigoloid arro/d neair u)c 4d( n,asnoitaredisn olcamre hrt of
m ireta noitatropsna r et. heTm i ftsodoir egpn orlet ftanemnorivne/dnuo reg hott ndiesael e er obdtemus ssala
of radio y lye tt o iae d telm g enrevi isaetaolicmterhstbtaaoltotacac fnruitwavaoif sseetfm riierrhtetetrni l
repositor y se vyl l or.l5 vosaentecmic miiaoapt etryrft - e0fsc5o rn -eaOethetutys o adsweic anlip aanif l
01 edulcni tseretni fo semarf emirt ,yrotisope snoitaredisn ogcnita erh oefruso lycrotisop erret fsara e0y00 ,o1t
etfa sraaey 000,01 ot 000,1 dn r o .Ftnemnorivn eeh to tstimi lesaele revitalumu cdn asleve leiru cro ferusol cr
1
tahwemos era tseretni fo semarf emit eht ,snreccnoc ytilacitir -fla heva hsepotos ielissi flapicnir peh tecni snep o
0 1f oredr oeh tn osevil 8 .sraey
Each r ev ietpcoatoois disaah ,atenf eirlhe-cffiflhiaw dhnac tfihs e echetvniattarlo epfrmoicae h
ol eht revio epotos o tsdee nydut sgnikna redilcu nasu h .Tngise dyrotisope reh to tnrecno cf osdoire pemi tgn
yaced evitcaoidar taht tcecffe eht redisno ta e,hytilaciti r,cgnidleihs—ae rsaisyla nhac are ogfnikn aer h ntsoah
tfsnar noitadila vdeliate dro fwoll adluoh ssgnikna rese h .T)yticixo tlacigoloidar (eso dlatnemnorivn edn a,re
necnoc eb ot stroffe tnemaevorpmi atad dn tnacifingi saeva hya mtah tsedilcu nf orebmu ndetimi leh tn odetart
.sevitcejb oMWRC Oeh tf ostnemeriuqe rlanoitcnu feh tn otcapmi
mi edilcun sihtT fo tnempoleved eh LN R yOsbtrof fee h ftnooitaniml uec h sttirop egrnikn aercnatrop
acigoloidar puorG sresU BDC eht dna MWRCtO edivorp o sses s oastna eemvitatitna uhaqt iewettimmocb uls
(valida )et eht NEGIRO le ddoemidobme( ni 2NEGIRO dna,S-NEGIRO 4 eht ELA CmSe tnsoyissrevo f
.at acdipoto slianoitid dganiniat b foeocnatrop meivital eer hetgd u oj stlal e sw,a)NEGIRO
2